Estimativa indireta das emissões diárias de CO2 de energia fóssil a partir do NO2 do TROPOMI

  • role: First author第一作者
  • Affiliation:

    School of Environment Science and Spatial Informatics,China University of Mining and Technology, Xuzhou 221116, China

  • Email:lulingxiao@cumt.edu.cn
  • Introduction:E-maillulingxiao@cumt.edu.cn
LU Lingxiao1,  
  • role: Corresponding author通信作者
  • Affiliation:

    School of Environment Science and Spatial Informatics,China University of Mining and Technology, Xuzhou 221116, China

  • Email:qinkai@cumt.edu.cn
  • Introduction:E-mailqinkai@cumt.edu.cn
QIN Kai1*,  
  • Affiliation:

    School of Environment Science and Spatial Informatics,China University of Mining and Technology, Xuzhou 221116, China

COHEN Jason Blake1,  
  • Affiliation:

    School of Environment Science and Spatial Informatics,China University of Mining and Technology, Xuzhou 221116, China

LI Xiaolu1,  
  • Affiliation:

    Satellite Application Center for Ecology and Environment, Beijing 100094, China

ZHOU Chunyan2

Resumo

Para alcançar a meta de "duplo carbono", é crucial utilizar a tecnologia de sensoriamento remoto por satélite para estimar as emissões de dióxido de carbono (CO2) provenientes do consumo de energia fóssil. No entanto, devido à longa vida útil do CO2 na atmosfera e à cobertura espacial limitada dos sensores de CO2 existentes por satélite, é difícil estimar diretamente as emissões a partir dos dados de concentração de coluna de CO2 invertidos das observações satelitais. Considerando que o consumo de energia fóssil emite simultaneamente CO2 e óxidos de nitrogênio (NOx), sendo o NOx de curta duração e com boa viabilidade para estimar suas emissões via sensoriamento remoto por satélite, este estudo selecionou 28 cidades do leste e uma região do triângulo dourado de energia do oeste para realizar um estudo de estimativa indireta das emissões diárias de CO2 baseadas na concentração de coluna de NO2 do TROPOMI. Primeiramente, utilizaram-se os dados da concentração da coluna troposférica de NO2 do TROPOMI de 2019 e um modelo de conservação de massa para estimar as emissões diárias de NOx e sua incerteza. Em seguida, analisou-se a relação entre as emissões de CO2 e NOx no banco de dados do inventário de emissões construído pelo modelo de inventário multiescalar (MEIC). Por fim, estimaram-se as emissões diárias de CO2 provenientes do consumo de energia fóssil. Os resultados mostram que as estimativas coincidem com a distribuição espacial das emissões de CO2 no inventário MEIC, mas sua maior resolução espacial e frequência temporal possibilitam revelar fontes de emissão emergentes e pequenas devido à falta de dados estatísticos. Nas cidades do leste, como Pequim, as estimativas por sensoriamento remoto nas áreas suburbanas ao redor do centro da cidade são cerca de 104% maiores do que o inventário MEIC, indicando o surgimento de várias fontes de emissão emergentes com a rápida expansão dessas cidades. No triângulo dourado de energia, exemplificado por Yulin, algumas fontes de emissão em usinas de energia, siderúrgicas e áreas de minas representam apenas 10% do total do inventário MEIC, enquanto a estimativa atribui 37%, indicando que pequenas usinas e fontes industriais não incluídas no inventário podem ser detectadas pelo sensoriamento remoto por satélite. Os resultados da pesquisa podem fornecer suporte técnico para a contabilização das emissões de carbono provenientes do consumo de energia fóssil na China.

Palavras-chave

sensoriamento remoto;energia fóssil;óxidos de nitrogênio;dióxido de carbono;TROPOMI;inventário de emissões;estimativa indireta;conservação de massa;fontes emergentes de emissão

References

  1. 1.
    Akimoto H, Ohara T, Kurokawa J I and Horii N. 2006. Verification of energy consumption in China during 1996-2003 by using satellite observational data. Atmospheric Environment, 40(40): 7663-7667
  2. 2.
    Berezin E V, Konovalov I B, Ciais P, Richter A, Tao S, Janssens-Maenhout G, Beekmann M and Schulze E D. 2013. Multiannual changes of CO2 emissions in China: indirect estimates derived from satellite measurements of tropospheric NO2 columns. Atmospheric Chemistry and Physics, 13(18): 9415-9438
  3. 3.
    Brasseur G P and Jacob D J. 2017. Modeling of Atmospheric Chemistry. Cambridge: Cambridge University Press
  4. 4.
    Canadell J G, Le Quéré C, Raupach M R, Field C B, Buitenhuis E T, Ciais P, Conway T J, Gillett N P, Houghton R A and Marland G. 2007. Contributions to accelerating atmospheric CO2 growth from economic activity, carbon intensity, and efficiency of natural sinks. Proceedings of the National Academy of Sciences of the United States of America, 104(47): 18866-18870
  5. 5.
    Ciais P, Dolman A J, Bombelli A, Duren R, Peregon A, Rayner P J, Miller C, Gobron N, Kinderman G, Marland G, Gruber N, Chevallier F, Andres R J, Balsamo G, Bopp L, Bréon F M, Broquet G, Dargaville R, Battin T J, Borges A, Bovensmann H, Buchwitz M, Butler J, Canadell J G, Cook R B, Defries R, Engelen R, Gurney K R, Heinze C, Heimann M, Held A, Henry M, Law B, Luyssaert S, Miller J, Moriyama T, Moulin C, Myneni R B, Nussli C, Obersteiner M, Ojima D, Pan Y, Paris J D, Piao S L, Poulter B, Plummer S, Quegan S, Raymond P, Reichstein M, Rivier L, Sabine C, Schimel D, Tarasova O, Valentini R, Wang R, Van Der werf G, Wickland D, Williams M and Zehner C. 2014. Current systematic carbon-cycle observations and the need for implementing a policy-relevant carbon observing system. Biogeosciences, 11(13): 3547-3602
  6. 6.
    Eldering A, Wennberg P O, Crisp D, Schimel D S, Gunson M R, Chatterjee A, Liu J, Schwandner F M, Sun Y, O’dell C W, Frankenberg C, Taylor T, Fisher B, Osterman G B, Wunch D, Hakkarainen J, Tamminen J and Weir B. 2017. The orbiting carbon observatory-2 early science investigations of regional carbon dioxide fluxes. Science, 358(6360): eaam5745
  7. 7.
    Goldberg D L, Lu Z F, Oda T, Lamsal L N, Liu F, Griffin D, McLinden Chris A, Krotkov N A, Duncan B N and Streets D G. 2019. Exploiting OMI NO2 satellite observations to infer fossil-fuel CO2 emissions from U.S. megacities. Science of the Total Environment, 695: 133805
  8. 8.
    Guan D B, Liu Z, Geng Y, Lindner S and Hubacek K. 2012. The gigatonne gap in China’s carbon dioxide inventories. Nature Climate Change, 2(9): 672-675
  9. 9.
    Hakkarainen J, Ialongo I, Oda T, Szeląg M E, O’Dell C W, Eldering A and Crisp D. 2023. Building a bridge: characterizing major anthropogenic point sources in the South African Highveld region using OCO-3 carbon dioxide snapshot area maps and Sentinel-5P/TROPOMI nitrogen dioxide columns. Environmental Research Letters, 18(3): 035003
  10. 10.
    Hakkarainen J, Ialongo I and Tamminen J. 2016. Direct space‐based observations of anthropogenic CO2 emission areas from OCO‐2. Geophysical Research Letters, 43(21): 11400-11406
  11. 11.
    Hammerling D M, Michalak A M, O’Dell C and Kawa S R. 2012. Global CO2 distributions over land from the Greenhouse Gases Observing Satellite (GOSAT). Geophysical Research Letters, 39(8): L08804
  12. 12.
    IPCC. 2014. Climate change 2014: impacts, adaptation, and vulnerability. Part A: global and sectoral aspects. IPCC
  13. 13.
    Janssens-Maenhout G, Crippa M, Guizzardi D, Muntean M, Schaaf E, Dentener F, Bergamaschi P, Pagliari V, Olivier J G J, Peters J A H W, Van Aardenne J A, Monni S, Doering U, Petrescu A M R, Solazzo E and Oreggioni G D. 2019. EDGAR v4.3.2 Global Atlas of the three major greenhouse gas emissions for the period 1970-2012. Earth System Science Data, 11(3): 959-1002
  14. 14.
    Konovalov I B, Berezin E V, Ciais P, Broquet G, Beekmann M, Hadji-Lazaro J, Clerbaux C, Andreae M O, Kaiser J W and Schulze E D. 2014. Constraining CO2 emissions from open biomass burning by satellite observations of co-emitted species: a method and its application to wildfires in Siberia. Atmospheric Chemistry and Physics, 14(19): 10383-10410
  15. 15.
    Konovalov I B, Berezin E V, Ciais P, Broquet G, Zhuravlev R V and Janssens-Maenhout G. 2016. Estimation of fossil-fuel CO2 emissions using satellite measurements of “proxy” species. Atmospheric Chemistry and Physics, 16(21): 13509-13540
  16. 16.
    Korsbakken J I, Peters G P and Andrew R M. 2016. Uncertainties around reductions in China’s coal use and CO2 emissions. Nature Climate Change, 6(7): 687-690
  17. 17.
    Kort E A, Frankenberg C, Miller C E and Oda T. 2012. Space‐based observations of megacity carbon dioxide. Geophysical Research Letters, 39(17): L17806
  18. 18.
    Li M, Liu H, Geng G N, Hong C P, Liu F, Song Y, Tong D, Zheng B, Cui H Y, Man H Y, Zhang Q and He K B. 2017a. Anthropogenic emission inventories in China: a review. National Science Review, 4(6): 834-866
  19. 19.
    Li M, Zhang Q, Kurokawa J I, Woo J H, He K B, Lu Z F, Ohara T, Song Y, Streets D G, Carmichael G R, Cheng Y F, Hong C P, Huo H, Jiang X J, Kang S C, Liu F, Su H and Zheng B. 2017b. MIX: a mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP. Atmospheric Chemistry and Physics, 17(2): 935-963
  20. 20.
    Li X L, Cohen J B, Qin K, Geng H, Wu X H, Wu L L, Yang C L, Zhang R and Zhang L Q. 2023. Remotely sensed and surface measurement-derived mass-conserving inversion of daily NOx emissions and inferred combustion technologies in energy-rich northern China. Atmospheric Chemistry and Physics, 23(14): 8001-19
  21. 21.
    Liu F, Duncan B N, Krotkov N A. , Lamsal L N, Beirle S, Griffin D, McLinden C A, Goldberg D L and Lu Z F. 2020. A methodology to constrain carbon dioxide emissions from coal-fired power plants using satellite observations of co-emitted nitrogen dioxide. Atmospheric Chemistry and Physics, 20(1): 99-116
  22. 22.
    Nassar R, Hill T G, McLinden C A, Wunch D, Jones D B A and Crisp D. 2017. Quantifying CO2 emissions from individual power plants from space. Geophysical Research Letters, 44(19): 10045-10053
  23. 23.
    Oda T, Bun R, Kinakh V, Topylko P, Halushchak M, Marland G, Lauvaux T, Jonas M, Maksyutov S, Nahorski Z, Lesiv M, Danylo O and Horabik-Pyzel J. 2019. Errors and uncertainties in a gridded carbon dioxide emissions inventory. Mitigation and Adaptation Strategies for Global Change, 24(6): 1007-1050
  24. 24.
    Qin K, Lu L X, Liu J, He Q, Shi J C, Deng W Z, Wang S and Cohen J B. 2023. Model-free daily inversion of NOx emissions using TROPOMI (MCMFE-NOx) and its uncertainty: declining regulated emissions and growth of new sources. Remote Sensing of Environment, 295: 113720
  25. 25.
    Reuter M, Buchwitz M, Hilboll A, Richter A, Schneising O, Hilker M, Heymann J, Bovensmann H and Burrows J P. 2014. Decreasing emissions of NOx relative to CO2 in East Asia inferred from satellite observations. Nature Geoscience, 7(11): 792-795
  26. 26.
    Schwandner F M, Gunson M R, Miller C E, Carn S A, Eldering A, Krings T, Verhulst K R, Schimel D S, Nguyen H M, Crisp D, O’dell C W, Osterman G B, Iraci L T and Podolske J R. 2017. Spaceborne detection of localized carbon dioxide sources. Science, 358(6360): eaam5782
  27. 27.
    Solazzo E, Crippa M, Guizzardi D, Muntean M, Choulga M and Janssens-Maenhout G. 2021. Uncertainties in the Emissions Database for Global Atmospheric Research (EDGAR) emission inventory of greenhouse gases. Atmospheric Chemistry and Physics, 21(7): 5655-5683
  28. 28.
    Van Geffen J, Boersma K F, Eskes H, Sneep M, Ter Linden M, Zara M and Veefkind J P. 2020. S5P TROPOMI NO2 slant column retrieval: method, stability, uncertainties and comparisons with OMI. Atmospheric Measurement Techniques, 13(3): 1315-1335
  29. 29.
    Veefkind J P, Aben I, McMullan K, Förster H, De Vries J, Otter G, Claas J, Eskes H J, De Haan J F, Kleipool Q, Van Weele M, Hasekamp O, Hoogeveen R, Landgraf J, Snel R, Tol P, Ingmann P, Voors R, Kruizinga B, Vink R, Visser H and Levelt P F. 2012. TROPOMI on the ESA Sentinel-5 Precursor: a GMES mission for global observations of the atmospheric composition for climate, air quality and ozone layer applications. Remote Sensing of Environment, 120: 70-83
  30. 30.
    Wang Y L, Broquet G, Ciais P, Chevallier F, Vogel F, Kadygrov N, Wu L, Yin Y, Wang R and Tao S. 2017. Estimation of observation errors for large-scale atmospheric inversion of CO2 emissions from fossil fuel combustion. Tellus B: Chemical and Physical Meteorology, 69(1): 1325723
  31. 31.
    Wheeler D and Ummel K. 2008. Calculating carma: global estimation of CO2 emissions from the power sector. SSRN Electronic Journal
  32. 32.
    Wu D E, Lin J C, Fasoli B, Oda T, Ye X X, Lauvaux T, Yang E G and Kort E A. 2018. A Lagrangian approach towards extracting signals of urban CO2 emissions from satellite observations of atmospheric column CO2 (XCO2): X-Stochastic Time-Inverted Lagrangian Transport model (“X-STILT v1”). Geoscientific Model Development, 11(12): 4843-4871
  33. 33.
    Yang E G, Kort E A, Ott L E, Oda T and Lin J C. 2023. Using space‐based CO2 and NO2 observations to estimate urban CO2 emissions. Journal of Geophysical Research: Atmospheres, 128(6): e2022JD037736
  34. 34.
    Zheng B, Geng G N, Ciais P, Davis S J, Martin R V, Meng J, Wu N N, Chevallier F, Broquet G, Boersma F, Van Der A R, Lin J T, Guan D B, Lei Y, He K B and Zhang Q. 2020. Satellite-based estimates of decline and rebound in China’s CO2 emissions during COVID-19 pandemic. Science Advances, 6(49): eabd4998
  35. 35.
    Zheng B, Tong D, Li M, Liu F, Hong C P, Geng G N, Li H Y, Li X, Peng L Q, Qi J, Yan L, Zhang Y X, Zhao H Y, Zheng Y X, He K B and Zhang Q. 2018. Trends in China’s anthropogenic emissions since 2010 as the consequence of clean air actions. Atmospheric Chemistry and Physics, 18(19): 14095-14111

Leia o texto completo

The above content is generated by Large Model Translation. The translated content is for reference only. We do not assume any commercial or legal responsibilty for any consequences arising from the use of our website